Nonlinear X-Ray Spectroscopy for Materials Science (Springer Series in Optical Sciences, 246)

Preface
Contents
Contributors
Abbreviations
1 Introduction
	1.1 Nonlinearity
	1.2 Classical Model of Nonlinear Optical Process
	1.3 Pragmatic Importance of Nonlinear Spectroscopy for Materials Science
	1.4 Synopsys
	Bibliography
2 Linear X-Ray Spectroscopy
	2.1 Basics
		2.1.1 Optical Responses of Materials in the X-Ray Region
		2.1.2 X-Ray Sources
		2.1.3 Light–Matter Interactions
	2.2 X-Ray Spectroscopy
		2.2.1 X-Ray Absorption Spectroscopy
		2.2.2 Photoelectron Spectroscopy
		2.2.3 X-Ray Emission Spectroscopy
	2.3 Time-Resolved X-Ray Spectroscopy
		2.3.1 Measurement Principles
		2.3.2 Examples of Time-Resolved Photoemission Spectroscopy Measurement
	2.4 Researcher’s Guide to Material Characterization with X-Rays
		2.4.1 The Guiding Chart for Experiments
		2.4.2 Application for Beamtime at the X-Ray Facility
	2.5 Summary
	References
3 Probing Nonlinear Light–Matter Interaction in Momentum Space: Coherent Multiphoton Photoemission Spectroscopy
	3.1 Introduction
	3.2 Experimental Setup
		3.2.1 Experimental Setup: The Photoelectron Analyzer
		3.2.2 Experimental Setup: The Light-Source
	3.3 mPP: Highly Nonlinear Mapping of the Energy- and Momentum-Dispersive Electronic Band Structure
		3.3.1 Static mPP in Threshold Order of Photoemission
		3.3.2 Above Threshold Photoemission
		3.3.3 Toward Full Surface Brillouin Zone Mapping by Coherent mPP
	3.4 Coherent Two-Dimensional Photoelectron Spectroscopy
		3.4.1 Coherent 2D FT Photoelectron Spectroscopy—Optical Bloch Equation Modeling
		3.4.2 Coherent 2D FT Photoelectron Spectroscopy of Ag(111)
		3.4.3 Coherent Above Threshold Photoemission
	3.5 Ultrafast Quasiparticle Dressing by Light
	3.6 Conclusion
	References
4 Nonlinear Soft X-Ray Spectroscopy
	4.1 Nonlinear Spectroscopy—Development with Visible Light
	4.2 Ultrafast X-Ray Light Sources
	4.3 Family of Soft X-Ray Nonlinear Spectroscopy
	4.4 Nonlinear Soft X-Ray Optics and Spectroscopies
		4.4.1 Multiphoton Absorption
		4.4.2 Stimulated Emission/Forward Scattering
		4.4.3 Stimulated Raman Scattering
		4.4.4 Four Wave Mixing
		4.4.5 Soft X-Ray Second Harmonic Generation/Sum Frequency Generation
	4.5 Theoretical Calculations for the Spectral Analysis
	4.6 Summary
	References
5 Nonlinear X-Ray Spectroscopy
	5.1 Introduction
	5.2 The Basic Theory of Nonlinear Optics in the Hard X-Ray Region
		5.2.1 Nonlinear Polarizability
		5.2.2 X-Ray Second Harmonic Generation
		5.2.3 Parametric Down-Conversion
		5.2.4 Sum Frequency Generation
	5.3 Featuring Examples of Nonlinear X-Ray Spectroscopy
		5.3.1 X-Ray Two-Photon Absorption Spectroscopy
		5.3.2 Saturable Absorption
		5.3.3 Atomic X-Ray Laser
		5.3.4 Stimulated X-Ray Emission Spectroscopy
		5.3.5 X-Ray Transient Grating Spectroscopy
	5.4 Summary
	References
6 Future Prospects
	6.1 Toward Multi-dimensional Spectroscopy
	6.2 Phase Sensitive Spectroscopy
	6.3 Vacuum Nonlinear X-Ray Optics
	6.4 Developments in Experimental Stations for Materials Science
	6.5 Into the Deep: Nonlinear Science
	References
Index