New Developments in Selective Oxidation II, Proceedings of the Second World Congress and Fourth European Workshop Meeting

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Page iii

Copyright page
Page iv

Preface
Pages v-vi
V. Cortés Corberán, S. Vic Bellón

Organization
Pages vii-viii

Modelling of propylene oxidation in a circulating fluidized-bed reactor Original Research Article
Pages 1-18
G.S. Patience, P.L. Mills

Selective oxidation over structured multicomponent molybdate catalysts Original Research Article
Pages 19-30
Joe Y. Zou, Glenn L. Schrader

Relationships between the catalytic activity and the composition of various uranium-antimony mixed oxide catalysts in the selective oxidation of olefins Original Research Article
Pages 31-40
F. Gama Freire, J.M. Herrmann, M.F. Portela

Synergy in the Fe-Mo-Sb-O Multiphase System Original Research Article
Pages 41-54
L.E. Cadus, Y.L. Xiong, F.J. Gotor, D. Acosta, J. Naud, P. Ruiz, B. Delmon

Role of Tellurium Oxide in the Selective Oxidation of Isobutene to Methacrolein: α-Sb2O4—TeO2 Catalysts Original Research Article
Pages 55-66
P. Oelker, L. Cadus, D. Forget, L. Daza, C. Papadopoulou, F. Gil Llambias, J. Naud, P. Ruiz, B. Delmon

Propylene Selective Oxidation as Studied by Oxygen-18 Labelling on Well-Denned MoO3 Catalysts Original Research Article
Pages 67-74
M. Abon, M. Roullet, J. Massardier, P. Delichère, A. Guerrero-Ruiz

Selective Hydrocarbon Oxidation at Vanadium Pentoxide Surfaces: Ab Initio Cluster Model Studies Original Research Article
Pages 75-81
Malgorzata Witko, Klaus Hermann

Comparison between gamma-alumina and aluminum niobate supported vanadium oxides in propane oxidative dehydrogenation Original Research Article
Pages 83-92
J.-G. Eon, P.G. Pries de Oliveira, F. Lefebvre, J.-C. Volta

Dispersion of V4+ ions in a SnO2 rutile matrix as a tool for the creation of active sites in ethane oxydehydrogenation Original Research Article
Pages 93-102
S. Bordoni, F. Castellani, F. Cavani, F. Trifirò, M.P. Kulkarni

Oxidative dehydrogenation of ethane over chromia-pillared montmorillonite catalysts Original Research Article
Pages 103-111
P. Olivera-Pastor, J. Maza-Rodrfguez, A. Jiménez-López, I. Rodriguez-Ramos, A. Guerrero-Rufz, J.L.G. Fierro

Oxidative dehydrogenation of propane and n-butane on V-Mg based catalysts Original Research Article
Pages 113-123
A. Corrna, J.M López Nieto, N. Parades, A. Dejoz, I. Vazquez

Oxidative Dehydrogenation of The C4-C5 Paraffins Over Vanadium-Containing Oxide Catalysts Original Research Article
Pages 125-132
R.G. Rizayev, R.M. Talyshinskii, J.M. Seifullayeva, E.M. Guseinova, Yu.A. Panteleyeva, E.A. Mamedov

Oxidehydrogenation of propane on gallium oxide-faujasite catalysts Original Research Article
Pages 133-142
B. Sulikowski, J. Kryściak, R.X. Valenzuelab, V. Cortés Corberán

Characteristics of alumina boria catalysts used in ethane partial oxidation Original Research Article
Pages 143-149
G. Cucinieri Colorio, B. Bonnetotb, J.C. Vedrine, A. Auroux

Effect of Potassium Addition to V2O5/TiO2 and MoO3/TiO2 Catalysts on Their Physicochemical and Catalytic Properties in Oxidative Dehydrogenation of Propane Original Research Article
Pages 151-158
B. Grzybowska, P. Mekšs, R. Grabowski, K. Wcisto, Y. Barbaux, L. Gengembre

Catalytic Reduction of Carbon Dioxide by Hydrocarbons and Other Organic Compounds Original Research Article
Pages 159-166
O.V. Krylov, A.Kh. Mamedov, S.R. Mirzabekova

A Concise Description of the Bulk Structure of Vanadyl Pyrophosphate and Implications for n-Butane Oxidation Original Research Article
Pages 167-181
Michael R. Thompson, A.C. Hessa, J.B. Nicholas, J.C. Whitea, J. Anchell, J.R. Ebnerb

A study of the (surface) structure of V-P-O catalysts during pretreatment and during activation Original Research Article
Pages 183-193
R.A. Overbeek, M. Versluijs-Helder, P.A. Warringa, E.J. Bosma, J.W. Geus

The Oxidation of n-Butane on Vanadyl Pyrophosphate Catalysts: Study of the Pretreatment Process Original Research Article
Pages 195-202
B. Kubias, M. Meisel, G.U. Wolf, U. Rodemerck

Activation of Vanadium Phosphorus Oxide Catalysts for Alkane Oxidation Oxygen Storage and Catalyst Performance Original Research Article
Pages 203-212
Y. Schuurman, J.T. Gleaves, J.R. Ebner, M.J. Mummey

Vanadium Phosphate Catalysts Prepared by the Reduction of VOPO4, 2H20 Original Research Article
Pages 213-220
Graham J. Hutchings, René Olier, Maria Teresa Sananés, Jean-Claude Volta

Production of Maleic and Phthalic Anhydrides by Selective Vapor Phase Oxidation with Vanadium Oxide Based Catalysts Original Research Article
Pages 221-231
C. Fumagalli, G. Golinelli, G. Mazzoni, M. Messori, G. Stefani, F. Trifirò

A New Commercial Scale Process for n-Butane Oxidation to Maleic Anhydride Using a Circulating Fluidized Bed Reactor Original Research Article
Pages 233-242
R.M. Contractor, D.I. Garnett, H.S. Horowitz, H.E. Bergna, G.S. Patience, J.T. Schwartz, G.M. Sisler

Separation of Catalyst Oxidation and Reduction—An Alternative to the conventional Oxidation of n-Butane to Maleic Anhydride? Original Research Article
Pages 243-251
G. Emig, K. Uihlein, C.-J. Häcker

On the catalyst features affecting selectivity in n-C4 hydrocarbon oxidation and oxidative dehydrogenation. Ft-IR studies Original Research Article
Pages 253-263
G. Busca, V. Lorenzelli, G. Oliveri, G. Ramis

New reaction: n-Butane direct catalytic oxidation to tetrahydrofuran Original Research Article
Pages 265-270
V.A. Zazhigalov, J. Habei, J. Stoch, G.A. Komashko, A.I. Pyatnitskaya, I.V. Bacherikova

Oxidation and ammoxidation of propane over tetragonal type M5+OPC4 catalysts Original Research Article
Pages 271-279
Ikuya Matsuura, Naomasa Kimura

Structure and Stability during the Catalytic Reaction of Unsupported V-Antimonate Catalysts for the Direct Selective Ammoxidation of Propane to Acrylonitrile Original Research Article
Pages 281-292
Gabriele Centi, Elisabetta Foresti, Francesco Guarnieri

Ammoxidation of propane over vanadium-antimony-oxide catalysts. Role of phase cooperation effects Original Research Article
Pages 293-303
R. Nilsson, T. Lindblad, A. Andersson, C. Song, S. Hansen

Selective oxidation of propane in the presence of bismuth-based catalysts Original Research Article
Pages 305-314
J Barrault, L Magaud, M. Ganne, M Toumoux

A Study of the Catalytic Oxidative Oligomerization of Methane to Aromatics Original Research Article
Pages 315-326
Andrew P.E. York, John B. Claridge, Malcolm L.H. Green, Shik Chi Tsang

Investigation of Molten Cobalt Halide/Sodium Metavanadate Mixtures as Redox Catalysts for the Oxidative Coupling of Methane Original Research Article
Pages 327-335
J.B. Claridge, M.L.H. Green, R.M. Lago, S.C. Tsang, A.P.E. York

The Active Oxygen Species in Oxidative Coupling of Methane Over Li/CaO and Na/CaO USING N2O and O2 as Oxidants Original Research Article
Pages 337-344
A.G. Anshits, V.G. Roguleva, E.V. Kondratenko

Spectroscopic Characterization of Surface Oxygen Species on Barium-Containing Methane Coupling Catalysts Original Research Article
Pages 345-356
Michael P. Rosynek, Dhammike Dissanayake, Jack H. Lunsford

Selectivity Control by Oxygen Pressure in Methane Oxidation Over Phosphate Catalysts Original Research Article
Pages 357-365
M. Yu. Sinev, S. Setiadi, K. Otsuka

Isotopic Labeling Studies on Oxidative Coupling of Methane over Alkali Promoted Molybdate Catalysts Original Research Article
Pages 367-375
S.A. Driscoll, U.S. Ozkan

Methane Coupling Over Sm-Al Mixed Oxides Original Research Article
Pages 377-385
P. Malet, M.J. Capitan, M.A. Centeno, J.J. Benitez, I. Carrizosa, J.A. Odriozola

Catalytic Reactor Engineering for the Oxidative Coupling of Methane. Use of a Fluidized Bed and of a Ceramic Membrane Reactor Original Research Article
Pages 387-394
A. Santos, C. Finol, J. Coronas, D. Lafarga, M. Menendez, J. Santamaría

Bi2O3-M2O3 Catalysts for Oxidative Coupling of Methane: Relationship between Structural Features and Catalytic Behaviours Original Research Article
Pages 395-401
E.A. Mamedov, N.T. Shamilov, V.P. Vislovskii, P.N. Joshi, S. Badrinarayan

Oxidative Conversion of Methane Over MgO/ZSM-5 Catalysts Original Research Article
Pages 403-409
P. Kovacheva, N. Davidova, A.H. Weiss

Surface characterization and catalytic behaviour of Li/MgO in oxidative coupling of methane Original Research Article
Pages 411-418
C.L. Padró, W.E. Grosso, G.T. Baronetti, A.A. Castro, O.A. Scelza

Solid—Gas Phase Interface Analysis on ZrO2: Correlation between CH4 Oxidation Activity and Work Function Measurements Original Research Article
Pages 419-426
D. Bouqueniaux, L. Jalowiecki-Duhamel, Y. Barbaux

The Rôle of Structural Defects and Oxygen Migration in La2O3 for the Oxidative Coupling of Methane Original Research Article
Pages 427-434
M.S. Islam, D.J. Ilett

Kinetic Simulation of Oxidative Coupling of Methane in the Gas Phase Original Research Article
Pages 435-441
V.I. Vedeneev, O.V. Krylov, V.S. Arutyunov, V. Ya. Basevich, M. Ya. Goldenberg, M.A. Teitel'boim

Oxidative Coupling of Methane over Ti-La-Na catalysts Original Research Article
Pages 443-450
S.T. Brandao, L. Lietti, P.L. Villa, S. Rossini, A. Santucci, R. Millini, O. Forlani, D. Sanfilippo

Gas Phase Oxidation of Benzene to Phenol using Pd/Cu Salt Catalysts: Effect of Counter Anion in Copper Salts Original Research Article
Pages 451-459
Kazuo Sasaki, Tomoyuki Kitano, Toshihiro Nakai, Miki Mori, Sotaro Ito, Masahiro Nitta, Katsuomi Takehira

Low Temperature Gas-Phase Selective Oxidation of 1-Butene to 2- Butanone on Supported Pd/V2O5 Catalysts Original Research Article
Pages 461-470
Gabriele Centi, Matteo Malaguti, Giuseppina Stella

The adsorption of oxygen on Ag and Ag-Au alloys: Mechanistic implications in ethylene epoxidation catalysis Original Research Article
Pages 471-480
Dimitris I. Kondarides, Xenophon E. Verykios

Detailed Modeling of Transport-Kinetics Interactions of Ethylene Epoxidation at High Vacuum and Atmospheric Pressures Original Research Article
Pages 481-493
G.D. Svoboda, J.T. Gleaves, P.L. Mills

Doping effects in ethylene epoxidation over potassium promoted silver catalysts Original Research Article
Pages 495-498
V. Lazarescu, M. Stanciu, M. Vass

A temperature programmed surface reaction study of the catalytic epoxidation and total oxidation of ethylene on silver Original Research Article
Pages 499-506
C. Henriques, M.F. Portela, C. Mazzocchia

HRTEM and TPO Study of the Behaviour under Oxidizing Conditions of some Rh/CeO2 Catalysts Original Research Article
Pages 507-514
S. Bernal, G. Blanco, J.J. Calvino, G.A. Cifredo, J. A. Pérez Omil, J.M. Pintado, A. Vara

Redox molecular sieves as heterogeneous catalysts for liquid phase oxidations Original Research Article
Pages 515-529
R.A. Sheldon, J.D. Chen, J. Dakka, E. Neeleman

Influence of the Synthesis Procedure and Chemical Composition on the Activity of Titanium in Ti-Beta Catalysts Original Research Article
Pages 531-540
M.A. Camblor, A. Corma, A. Martinez, J. Perez-Pariente, S. Valencia

Selective Oxidation of Ammonia to Hydroxylamine with Hydrogen Peroxide on Titanium Based Catalysts Original Research Article
Pages 541-550
M.A. Mantegazza, G. Leofanti, G. Petrini, M. Padovan, A. Zecchina, S. Bordiga

Palladium Catalyzed Oxidation of Benzene to Phenol Using Molecular Oxygen Original Research Article
Pages 551-559
Ulf Schuchardt, Alexandre T. Cruz, Luis C. Passoni, Carol H. Collins

Partial oxidation of cinnamyl alcohol on bimetallic catalysts of improved resistance to self-poisoning Original Research Article
Pages 561-570
T. Mallat, Z. Bodnar, M. Maciejewski, A. Baiker

Novel tungsten catalysts grafted onto polymeric materials: a comparison with phase transfer catalysis Original Research Article
Pages 571-581
J.-M. Brégeault, R. Thouvenot, S. Zoughebi, L Salles, A. Atlamsani, E. Duprey, C. Aubry, F. Robert, G. Chottard

Selective oxidation of cyclopentene and cyclohexene by hydrogen peroxide catalyzed by heteropolyacids Original Research Article
Pages 583-591
Kwan-Young Lee, Koshi Itoh, Masato Hashimoto, Noritaka Mizuno, Makoto Misono

Highly selective epoxidation of olefins on mono-transition-metal-substituted Keggin-type heteropolytungstates by molecular oxygen in the presence of aldehyde Original Research Article
Pages 593-601
N. Mizuno, T. Hirose, M. Iwamoto

Selective Oxidation of Cyclohexene with Molecular Oxygen Catalyzed by Transition Metal Substituted Polyoxometalates Original Research Article
Pages 603-608
Dujie Qin, Guojia Wang, Yue Wu

Novel Catalysts for Olefin Cleavage Using Hydrogen Peroxide Original Research Article
Pages 609-614
A. Johnstone, P.J. Middleton, W.R. Sanderson, M. Service, P.R. Harrison

Novel One-pot Synthesis of Indigo from Indole and Organic Hydroperoxide Original Research Article
Pages 615-622
Yoshihisa Inoue, Yoshihiro Yamamoto, Hiroharu Suzuki, Usaji Takaki

Selective Oxidations with Short-lived Manganese(V) Original Research Article
Pages 623-628
Éva Záhonyi-Budó, László I. Simándi

Catalytic Oxidation of Polyols: New Example of Nonradical Mechanism of Oxygenation Original Research Article
Pages 629-637
A.M. Sakharov, I.P. Skibida

Copper-catalyzed oxidative decarboxylation of aliphatic carboxylic acids Original Research Article
Pages 639-646
F.P.W. Agterberg, W.L. Driessen, J. Reedijk, H. Oeveringb, W. Buijs

Cyclohexane Oxidation by the Goagg111 System: Formation of Iron (HYDR)Oxide Particles and Reactivation Original Research Article
Pages 647-652
U. Schuchardt, C.E.Z. Krahembuhl, W.A. Carvalho

Oxidation of Cyclohexane Catalyzed by Polyhalogenated and Perhalogenated Manganese Porphyrins Original Research Article
Pages 653-658
P. Battioni, R. Iwanejkob, D. Mansuy, T. Mlodnicka

Polymer supported iron catalysts for the oxidation of cyclohexane Original Research Article
Pages 659-666
Ki-Won Jun, Eun-Kyung Shim, Seong-Bo Kim, Kyu-Wan Lee

Selective Oxidation of 2-Mercaptobenzothiazole Original Research Article
Pages 667-673
Milan Hronec, Magda Stolcova, Tibor Liptay

Selective Oxidation of Gaseous Hydrocarbons by Microbial Cells Original Research Article
Pages 675-683
G.A. Kovalenko, V.K. Sokolovskii

Selective Enzymatic Oxidations by using Oxygen as oxidizing agent: Immobilization and Stabilization of FNR, a NADP+ regenerating enzyme Original Research Article
Pages 685-692
T. Bes, R. Fernandez-Lafuente, C.M. Rosell, C. Gomez-Moreno, J.M. Guisan

ESR study of photo-oxidation of phenol at low temperature on polycrystalline titanium dioxide Original Research Article
Pages 693-701
M.J. López-Muñoz, J. Soria, J.C. Conesa, V. Augugliaro

Partial oxidation of benzene over the carbon whisker cathode added with iron oxide and palladium black during O2-H2 fuel cell reactions Original Research Article
Pages 703-711
Kiyoshi Otsuka, Mitsuhiro Kunieda, Ichiro Yamanaka

Influence of operational variables on the photodegradation kinetics of Monuron in aqueous titanium dioxide dispersions Original Research Article
Pages 713-720
V. Augugliaro, L. Cavallero, G. Marci, L. Palmisano, E. Pramauro

Heterogeneous Photocatalytic Oxidation of Liquid Isopropanol by TiO2, ZrO2 and ZrTiO4 Powders Original Research Article
Pages 721-728
J.A. Navio, G. Colón

Effect of the state of vanadium on the properties of titanium phosphate-based catalysts for oxidation of toluene Original Research Article
Pages 729-737
J. Soria, J.C. Conesa, V. Villalba, A. Aguilar Elguezabal, V.Cortes Corberan

Quantum—chemical description of the oxidation of alkylaromatic molecules on vanadium oxide catalysts Original Research Article
Pages 739-748
J. Haber, R. Tokarz, M. Witko

Characterisation of V2O5-Fe2O3-Cs2SO4 Catalysts for The Gas-Phase Oxidation of Fluorene to 9-Fluorenone Original Research Article
Pages 749-758
F. Majunke, S. Trautmann, M. Baerns

Gas-phase catalytic oxydehydrogenation of ethylbenzene on A1PO4 catalysts Original Research Article
Pages 759-768
F.M. Bautista, J.M. Campelo, A. Garcia, D. Luna, J.M. Marinas, R.A. Quiros

Selective gas-phase dehydrogenation of cyclohexanol with magnesium orthophosphates Original Research Article
Pages 769-776
M.A. Aramendia, J. Barrios, V. Borau, C. Jimenez, J.M. Marinas, F.J. Romero, J.R. Ruiz, F.J. Urbano

Effect of K-doping on 2-propanol adsorption, desorption and catalytic oxidation over vanadia-titania Original Research Article
Pages 777-785
G. Busca, V. Sanchez Escribano, P. Forzatti, L. Lietti, G. Ramis

Selective Oxidation of Methanol on Iron-Chromium-Molybdenum Oxide Catalysts Original Research Article
Pages 787-794
D. Klissurski, V. Rives, Y. Pesheva, I. Mitov, R. Stoyanova

Creation of New Selective Sites by Spill-Over Oxygen via α-Sb2O4 in the Oxidation of Ethanol Original Research Article
Pages 795-802
R. Castillo, P.A. Awasarkar, Ch. Papadopoulou, D. Acosta, P. Ruiz

Effect of titania on the properties of alumina supported molybdena catalysts Original Research Article
Pages 803-810
F. Requejo, N. Quaranta, J.M. Coronado, J. Soria, H. Thomas

Selective Dehydrogenation of Ethanol Over Vanadium Oxide Catalyst Original Research Article
Pages 811-818
N.E. Quaranta, R. Martino, L. Gambaro, H. Thomas

Cesium promotion of iron phosphate catalyst and influence of steam on the oxidative dehydrogenation of isobutyric acid to methacrylic acid Original Research Article
Pages 819-828
J. Belkouch, B. Taouk, L. Monceaux, E. Bordes, P. Courtine, G. Hecquet

Iron Hydroxysilicates: New Selective and Active Isobutyric Acid Oxidative Dehydrogenation Catalysts Original Research Article
Pages 829-835
P. Bonnet, J.M.M. Millet, J.C. Vedrine, G. Hecquet

Thermolysis of Heteropolyacid H3PMO12O40 and Catalytic Properties of the Thermal Decomposition Products in Oxidation of Acrolein to Acrylic Acid Original Research Article
Pages 837-844
T.V. Andrushkevich, V.M. Bondareva, R.I. Maksimovskaya, G. Ya. Popova, L.M. Plyasova, G.S. Litvak, A.V. Ziborov

Selective Oxidatioh of Aldehydes Over V-Mo-Ox/SiO2 Catalysts Original Research Article
Pages 845-852
J. Machek, J. àvachula, J. Tichy, L.J. Alemany, F. Delgado, J.M. Blasco

Diacetyl synthesis by the direct partial oxidation of methyl ethyl ketone over vanadium oxide catalysts Original Research Article
Pages 853-860
E. McCullagh, N.C. Rigas, J.T. Gleaves, B.K. Hodnett

Selective Oxidation of Hydrogen Sulfdde on A Sodium Promoted Dion Oxide on Silica Catalyst Original Research Article
Pages 861-868
R.J.A.M. Terörde, M.C. de Jong, M.J.D. Crombag, P.J. van den Brink, A.J. van Dillen, J.W. Geus

Effect of morphology of honeycomb SCR catalysts on the reduction of NOx and the oxidation of SO2 Original Research Article
Pages 869-876
A. Beretta, E. Tronconi, L.J. Alemany, J. Svachula, P. Forzatti

Author Index
Pages 877-880

Subject Index
Pages 881-884