New Aspects of Spillover Effect in Catalysis: For Development of Highly Active Catalysts: Proceedings of the Third International Conference on Spill

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Page iii

Copyright page
Page iv

Preface
Page v
Tomoyuki Inui, Kaoru Fujimoto, Toshio Uchijima, Mitsuo Masai

Organization: Organizing Committee
Page vi

The control of selectivity and stability of catalysts by spillover processes Original Research Article
Pages 1-8
Bernard Delmon

Catalyst design based on spillover theory Original Research Article
Pages 9-16
Kaoru Fujimoto

Spillover effect as the key concept for realizing rapid catalytic reactions Original Research Article
Pages 17-26
T. Inui

The history and perspectives of spillover Original Research Article
Pages 27-43
S.J. Teichner

Synergism in the catalysis of supported gold Original Research Article
Pages 45-52
M. Haruta, S. Tsubota, A. Ueda, H. Sakurai

The effect of spillover hydrogen on coke formation catalyzed by HY zeolite and pillared montmorillonite Original Research Article
Pages 53-60
E. Kikuchi, T. Matsuda

Spectroscopic insight into spillover Original Research Article
Pages 61-68
Wm. Curtis Conner Jr.

Molecular hydrogen-originated solid acid catalysts Original Research Article
Pages 69-76
Hideshi Hattori

Hydrocracking of residual oils with iron supported zeolite containing catalyst Original Research Article
Pages 77-84
Ikusei Nakamura, Ryuichiro Iwamoto, Akira I-ino

Attempt at the characterization of spillover adsorbed species during catalysis
Pages 85-93

Oxygen spillover for the design of industrial oxidation catalysts Original Research Article
Pages 95-103
Yoshihiko Moro-Oka

Surface-to-bulk spillover of hydrogen (proton) in the catalysis of solid heteropoly compounds Original Research Article
Pages 105-110
Makoto Misono, Hiroshi Igarashi, Koichi Katamura, Toshio Okuhara, Noritaka Mizuno

Ion spillover as the origin of the NEMCA effect Original Research Article
Pages 111-116
C.G. Vayenas, S. Bebelis, I.V. Yentekakis, S. Neophytides, Jiang Yi

Reduction of nitrous oxide by electrochemically-generated spillover hydrogen Original Research Article
Pages 117-123
Kiyoshi Otsuka, Hideaki Yamagata

Hydrogen spillover on bimetallic supported Pt-Re particles Original Research Article
Pages 125-130
Do Trong On, Michel Che, Laurent Bonneviot

The role of irreversible and reversible spillover hydrogen in reforming reactions Original Research Article
Pages 131-136
Songying Chen, Yuhan Sun, Shaoyi Peng

New experimental evidence of the long distance hydrogen back spillover (LD-HBS) mechanism in the paraffins aromatization on Zn and Ga ZSM catalysts Original Research Article
Pages 137-142
Gr. Pop, D. Ivanescu, R. Ganea

Hydrogen back spillover phenomena in the aromatization of light alkanes over hybrid catalysts. Mechanistic considerations Original Research Article
Pages 143-149
Raymond Le Van Mao, Jianhua Yao, Louise Dufresne, Riccardo Carli, Vittorio Ragaini

Hydrogen spillover in the conversion of cyclohexane on ZSM-5 zeolites Original Research Article
Pages 151-158
F. Roessner, U. Mroczek, A. Hagen

New active sltes induced by hydrogen spillover in reduced Pt-Ga/HZSM-5 aromatization catalysts Original Research Article
Pages 159-164
E.S. Shpiro, D.P. Shevchenko, R.V. Dmitriev, O.P. Tkachenko, Kh.M. Minachev

Hydroisomerization of n-pentane over hybrid catalysts containing supported hydrogenation catalyst Original Research Article
Pages 165-169
Kohjiroh Aimoto, Kaoru Fujimoto, Ken Maeda

The role of spillover in the hydrogenation of oxygenates adsorbed on Ni/Al2O3 Original Research Article
Pages 171-175
Baoshu Chen, John L. Falconer

Hydrogenation active sites of molybdenum sulfide catalysts enhanced by Ni and Co organometallics Original Research Article
Pages 177-182
Akio Nishijima, Suehiko Yoshitomi, Toshio Sato, Yuji Yoshimura, Hiromichi Shimada, Nobuyuki Matsubayashi

Electrical conductivity study of hydrogen spillover on TiO2 Original Research Article
Pages 183-188
Th. Braunschweig, U. Roland, H. Winkler

Direct observation of surface mobility with microscopic techniques Photoemission electron- and field electron microscopy Original Research Article
Pages 189-194
J.H. Block, M. Ehsasi, V. Gorodetskii, A. Karpowicz, M. Berdau

Selective hydrogen permeation through metal-dispersed porous alumina membrane Original Research Article
Pages 195-200
K. Eguchi, M.-R. Chai, Y. Yamashita, M. Machida, H. Arai

Surface migration of oxygen and of hydrogen in supported metal catalysts Original Research Article
Pages 201-206
D. Martin, D. Duprez

Catalysis and spillover Original Research Article
Pages 207-212
E.P.S. Barrett, A.J. Blackburn, M.A. Yates, Y. Wang, P.A. Sermon

Oxidative conversion of methane on Cu and Ag-NI electrodes at artificial unsteady-state mode of the SOFC reactor operation Original Research Article
Pages 213-216
V.D. Belyaev, V.A. Sobyanin, O.A. Marína

Spillover of atomic oxygen and reverse spillover of dioxygen species on Pt/CeO2 catalyst Original Research Article
Pages 217-222
Can Li, Yanxin Chen, Wenzhao Li, Qin Xin

Methoxy formation/spillover on Pd/Al2O3 studied by 13C, 1H NMR Original Research Article
Pages 223-228
Oc Hee Han, Gustavo Larsen, Kurt W. Zilm, Gary L. Haller

A surface structure model with allowance for spillover Original Research Article
Pages 229-234
R.K. Edvinsson, R.R. Hudgins, P.L. Silveston

A mathematical model for spillover Original Research Article
Pages 235-240
Y.W. Nam, P.L. Silveston

Promoting effect and hydrogen spillover in supported SeRh6-cluster catalysts Original Research Article
Pages 241-246
Y. Izumi, Y. Iwasawa

Heterogeneous catalytic ammoximation of cyclohexanone with ammonia and molecular oxygen Original Research Article
Pages 247-252
G. Busca, E. Giamello, D. Pinelli, F. Trifirò

CO chemisorption and CO-TPR in H2 stream with Rh/NaY and Rh-Zn/NaY zeolite catalysts Original Research Article
Pages 253-256
Y.-D. Xu, A.-M. Liu, D.-M. Li, J.-S. Huang, L. Huang

Plasma-induced chemisorption of nitrogen and hydrogen on alumina-supported platinum catalysts Original Research Article
Pages 257-260
S. Kameoka, S. Ito, K. Kunimori

Characterization of palladium catalyst supported on zeolite Original Research Article
Pages 261-264
Tokuo Matsuzaki, Koji Abe, Kyoji Ohdan, Shuji Tanaka, Keigo Nishihira, Asumaru Nakamura

Surface treatments of silica support for nickel catalyst: effects on hydrogen adsorption/desorption and ethane hydrogenolysis Original Research Article
Pages 265-268
M. Arai, K. Suzuki, Y. Nishiyama

Coadsorption of CO and NO on Co—Rh cluster—derived bimetallic catalysts and NO spillover phenomenon Original Research Article
Pages 269-272
Q. Xin, Z. Cao, Y.Q. Chen, Y. Chen, H. Zhang, C. Li

IR study of Rh-Sn bimetallic system and spillover of oxygen Original Research Article
Pages 273-276
S. Nishiyama, M. Akcmoto, I. Yamamoto, H. Yanagi, S. Tsuruya, M. Masai

Spillover to form CH3O on Pt/Al2O3 and Pd/La2O3 Original Research Article
Pages 277-280
Raymond L. Flesner, Keith B. Kester, Baoshu Chen, John L. Falconer

Nature of Brönsted-acid sites in Ag3PW12O40 in the presence of hydrogen and reversible interconversion of protons and hydrogen Original Research Article
Pages 281-284
Toshihide Baba, Mamoru Nomura, Yoichi Ohno, Yukiyo Hiroyama, Yoshio One

A new concept of hydrogen storage: a Pt/SO42 -ZrO2 material Original Research Article
Pages 285-288
Tsunehiro Tanaka, Kohki Ebitani, Hideshi Hattori, Satohiro Yoshida

Hydrogenation of isobutylene by spiltover hydrogen from Pt/KA-zeolite to NaY-zeolite Original Research Article
Pages 289-292
S. Ohgoshi, I. Nakamura, Y. wakushima

Influence of support modification on hydrogen spillover in ethylene hydrogenation over Pt/Al2O3 Catalyst Original Research Article
Pages 293-296
Genmin Lu

Hydrogenation of sodium fumarate in the solid phase over fine nickel powder Original Research Article
Pages 297-300
Tadao Harada, Tsutomu Osawa

New active site for CO hydrogenation formed on promoted Rh catalyst by spillover hydrogen Original Research Article
Pages 301-304
H. Kato, T. Mori, M. Nakajima, Y. Mori, T. Hattori, Y. Murakami

Spillover effect for the reducing reaction of CO2 with CH4 over SiO2-supported transition metal catalysts physically mixed with MgO Original Research Article
Pages 305-308
Osamu Takayasu, Naomi Hongo, Ikuya Matsuura

Acceleration of dehydrogenation reactions by hydrogen spillover Original Research Article
Pages 309-312
Hayao Imamura, Yoshihisa Sakata, Susurau Tsuchiya

Carbon-supported dehydrogenation catalysts composed of platinum and ruthenium metals Original Research Article
Pages 313-316
Yuji Ando, Xiaomei Li, Eri Ito, Masaru Yamashita, Yasukazu Saito

Diffusion of oxygen atoms from active sites during the catalytic oxidation of carbon monoxide with oxygen on molybdenum trioxide Original Research Article
Pages 317-320
Yasuo Iizuka

Spillover in catalyses over Co-phthalocyanines supported on titania Original Research Article
Pages 321-324
Isao Mochida, Takaaki Higashiizumi, Youichi Ishihara, Hiroshi Fujitsu

CO oxidation over gold supported on TiO2 Original Research Article
Pages 325-328
S. Tsubota, D. Cunningham, Y. Bando, M. Haruta

Platinum metals-ceria synergism in autoexhaust catalyst Original Research Article
Pages 329-332
T. Yamada, K. Kayano, M. Funabiki

Hysteresis and self-oscillation in a selective catalytic reduction of nitric oxide by hydrocarbons on alumina Original Research Article
Pages 333-336
A. Obuchi, A. Ogata, K. Mizuno, A. Ohi, H. Ohuchi

The effect of electrochemical pumping of oxygen on catalytic behaviour of metal electrodes in methane oxidation Original Research Article
Pages 337-340
O.A. Mar\'ina, V.A. Sobyanin, V.D. Belyaev, V.N. Parmon

Possibility of sulfur spillover on hydrodesulfurization catalysts using radioactive 35S Original Research Article
Pages 341-344
T. Kabe, A. Ishihara, W. Qian, S. Ogawa, H. Sakuno

New evidence of the promotion of activity and selectivity through hydrogen spill-over activation of biphasic sulfided hydrotreating catalysts Original Research Article
Pages 345-348
S. Giraldo de León, P. Grange, B. Delmon

Interaction between Co species and Mo species in C0O-M0O3/AI2o3 Original Research Article
Pages 349-352
Muneyoshi Yamada, Seiji Kasahara, Kan Kawahara

Hydrogen spillover on ruthenium promoted molybdenum catalysts for hydrodesulfurization Original Research Article
Pages 353-356
X.S. Li, Z.S. Hou, Q. Xin

Development of hydrodesulfurization catalysts prepared using metal carbonyls Original Research Article
Pages 357-360
A. Ishihara, M. Nomura, M. Azuma, M. Matsushita, K. Shirouchi, T. Kabe

Transfer hydrocracking of heavy oils with metal-supported carbon catalyst Original Research Article
Pages 361-364
Ikusei Nakamura, Kohjiro Aimoto, Kaoru Fujimoto

Enhancing effect of hydrogen sulfide for cracking of n-hexane over alkali and alkaline earth metal zeolites Original Research Article
Pages 365-368
M. Sugioka, M. Amisawa, K. Sato, H. Abe

Spillover effect in methane reforming reactions on Ni-based composite catalysts modified with precious metals Original Research Article
Pages 369-372
T. Inui, K. Fujioka, W. Tanakulrungsank, T. Takeguchi

Behavior of surface oxygen on a Rh/Si02 catalyst in oxidation of methane Original Research Article
Pages 373-376
J. Nakamura, K. Kubushiro, T. Uchijima

Utilization of oxide ion transfer for oxidative coupling of methane with membrane reactors Original Research Article
Pages 377-380
T. Nozaki, K. Omata, K. Fujimoto

Highly dispersed cobalt catalysts modified with transition metals and their applications to CO hydrogenation Original Research Article
Pages 381-384
Y. Sugi, T. Matsuzaki, H. Arakawa, K. Takeuchi, T. Hanaoka

Continuous catalysis on oxides in the presence of spiltover hydrogen Original Research Article
Pages 385-388
M.S.W. Vong, P.A. Sermon

Promoting effect of Ti02 addition to CuO-ZnO catalyst on methanol synthesis by catalytic hydrogenation of CO2 Original Research Article
Pages 389-392
H. Arakawa, K. Sayama, K. Okabe, A. Murakami

Spillover effect on the stabilization of Cu-Zn catalyst for CO2 hydrogenation to methanol Original Research Article
Pages 393-396
K. Fujimoto, Y. Yu

Hydrogenation of CO2 over metal supported fine particles Original Research Article
Pages 397-400
Takayoshi Uematsu, Masatoshi Fukuda, Tsuyoshi Iijima, Shogo Shimazu

Spillover effects of hydrogen on the reduction of CO2 over supported metal catalysts Original Research Article
Pages 401-404
Toshiaki Sodesawa, Satoshi Sato, Fumio Nozaki

Synergistic effect of Pd and Mn203 in combustion reactions Original Research Article
Pages 405-408
Y. Tsuji, S. Imamura

Catalytic gasification activity of iron enhanced by spilt-over hydrogen Original Research Article
Pages 409-412
Shiro Matsumoto, Sakumitsu Sakagami

Catalytic behavior of iron in the gasification of coal with hydogen Original Research Article
Pages 413-416
Kenji Asami, Yasuo Ohtsuka

Liquid-phase hydroxylation of xylene with hydrogen peroxide over zeolite catalysts Original Research Article
Pages 417-420
T. Yashima, S. Nagase, T. Komatsu, S. Nambab

Promoting effects of noble metals on the detection of ammonia by semiconductor gas sensor Original Research Article
Pages 421-424
Tomoki Maekawa, Jun Tamaki, Norio Miura, Noboru Yamazoe

Manganese oxide and niobium oxide catalysts prepared by a proton exchange and elimination method Original Research Article
Pages 425-428
Y. Inoue, K. Sato, H. Takahashi, S. Yasukawa

Promoting role of metal additives in modified Pd catalysts for selective hydrodechlorination of CFC-113 Original Research Article
Pages 429-432
R. Ohnishi, H. Suzuki, W.-L. Wang, M. Ichikawa

Author Index
Pages 433-435